Vol. 30, issue 01, article # 6

Sakerin S. M., Golobokova L. P., Kabanov D. M., Pol'kin V. V., Turchinovich Yu. S., Khodzher T. V., Khuriganova O. I. Spatiotemporal variations in aerosol characteristics along the route of the Indian-Atlantic expedition onboard RV “Akademik Nikolaj Strakhov”. // Optika Atmosfery i Okeana. 2017. V. 30. No. 01. P. 42-52. DOI: 10.15372/AOO20170106 [in Russian].
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Abstract:

We discuss the results of studying the physical-chemical composition of the atmospheric aerosol during expedition onboard RV “Akademik Nikolaj Strakhov” carried out during winter of 2015/2016 on the route from Colombo to Kaliningrad (via Suez Canal). In comparison with the Mediterranean Sea and Atlantic (near Europe), the atmosphere of the Arabian and Red Seas was characterized by higher values of most aerosol characteristics: 3–5 times larger aerosol optical depth (AOD), 4 times larger aerosol number concentration, 1.5 times larger concentrations of continent- and sea-derived ions, as well as more abundant gaseous admixtures (SO2, HCl, HNO3, NH3). At the same time, two seas of the Indian basin show substantial differences in aerosol composition, caused by outflows of aerosols of different types from the continents. The largest concentrations of black carbon (2.14 µg · m–3, on the average), sea-derived ions (Na+, Cl, Mg2+), and NH3 are observed over the Arabian Sea; and larger values of fine component of AOD and concentrations of “continental” ions (SO42–, Ca2+, NO3, NH4+) and gaseous admixtures SO2, HCl, HNO3 are found over the Red Sea. With respect to ion composition of aerosol, most stable concentrations are noted in Ca2+ ions (less than 15% difference among the seas), and maximal spatial variations are found in NH4+ ions (a difference is up to a factor of 40).

Keywords:

aerosol optical depth, aerosol and “black carbon” concentrations, chemical composition, Indian and Atlantic Ocean

References:

  1. Holben B.N., Eck T.F., Slutsker I., Tanre D., Buis J.P., Setzer A., Vermote E., Reagan J.A., Kaufman Y., Nakajima T., Lavenu F., Jankowiak I., Smirnov A. AERONET – A federated instrument network and data archive for aerosol characterization // Remote Sens. Environ. 1998. V. 66. P. 1–16.
  2. Issledovanie radiacionnyh harakteristik ajerozolja v aziatskoj chasti Rossii / Pod red. S.M. Sakerina. Tomsk: Izd-vo Instituta optiki atmosfery SO RAN, 2012. 484 p.
  3. Kuznecova I.N., Glazkova A.A., Shalygina I.Ju., Nahaev M.I., Arhangel'skaja A.A., Zvjagincev A.M., Semutnikova E.G., Zaharova P.V., Lezina E.A. Sezonnaja i sutochnaja izmenchivost' koncentracij vzveshennyh chastic v prizemnom vozduhe zhilyh rajonov Moskvy // Optika atmosf. i okeana. 2014. V. 27, N 6. P. 473–482.
  4. Arshinov M.Ju., Belan B.D., Davydov D.K., Ivlev G.A., Kozlov A.V., Kozlov A.S., Malyshkin S.B., Simonenkov D.V., Antohin P.N. Nukleacionnye vspleski v atmosfere boreal'noj zony Zapadnoj Sibiri. Part I. Klassifikacija i povtorjaemost' // Optika atmosf. i okeana. 2014. V. 27, N 9. P. 766–774.
  5. Gruzdev A.N., Isakov A.A. O prirode dolgoperiodnyh variacij massovoj koncentracii prizemnogo ajerozolja // Optika atmosf. i okeana. 2015. V. 28, N 9. P. 810–815; Gruzdev A.N., Isakov A.A. On the nature of long-period variations in mass concentration of near-ground aerosol // Atmos. Ocean. Opt. 2016. V. 29, N 1. P. 73–78.
  6. Smirnov A., Holben B.N., Kaufman Y.J., Dubovik O., Eck T.F., Slutsker I., Pietras C., Halthore R.N. Optical Properties of Atmospheric Aerosol in Maritime Environments // J. Atmos. Sci. 2002. V. 59, N 3. Pt. 1. P. 501–523.
  7. Sakerin S.M., Kabanov D.M., Smirnov A.V., Holben B.N. Aerosol optical depth of the atmosphere over ocean in the wavelength range 0.37–4 mm // Int. J. Remote Sens. 2008. V. 29, iss. 9. P. 2519–2547. DOI: 10.1080/01431160701767492.
  8. Smirnov A., Holben B.N., Slutsker I., Giles D., McClain C.R., Eck T.F., Sakerin S.M., Macke А., Croot P., Zibordi G., Quinn P., Sciare J., Kinne S., Harvey M., Smyth T., Piketh S., Zielinski T., Proshutinsky A., Goes J., Seigel D.A., Larouche P., Radionov V.F., Goloub P., Krishnamoorthy K., Matarrese R., Robertson L., Jourdin F. Maritime Aerosol Network as a component of Aerosol Robotic Network // J. Geoph. Res. 2009. V. 114. D06204. DOI: 10.1029/2008JD011257.
  9. Sakerin S.M., Bobrikov A.A., Bukin O.A., Golobokova L.P., Polkin Vas.V., Polkin Vik.V., Shmirko K.A., Kabanov D.M., Khodzher T.V., Onischuk N.A., Pavlov A.N., Potemkin V.L., Radionov V.F. On measurements of aerosol-gas composition of the atmosphere during two expeditions in 2013 along Northern Sea Route // Atmos. Chem. Phys. 2015. V. 15, iss. 21. P. 12413–12443. DOI: 10.5194/acp-15-1-2015.
  10. Tomasi C., Prodi F. Measurement of atmospheric turbidity and vertical mass loading of particulate matter in marine environments (Red Sea, Indian Ocean, and Somalian Coast) // J. Geophys. Res. C. 1982. V. 87, N 2. P. 1279–1286.
  11. Kedia S., Ramachandran S. Variability in aerosol optical and physical characteristics over the Bay of Bengal and the Arabian Sea deduced from Angstrem exponents // J. Geophys. Res. 2009. V. 114. D14207. DOI: 10.1029/2009JD011950.
  12. Kalapureddy M.C.R., Kaskaoutis D.G., Raj P.E., De-vara P.C.S., Kambezidis H.D., Kosmopoulos P.G., Nas-tos P.T. Identification of aerosol type over the Arabian Sea in the premonsoon season during the Integrated Campaign for Aerosol, Gases and Radiation Budget (ICARB) // J. Geophys. Res. 2009. V. 114. D17203. DOI: 10.1029/2009JD011826.
  13. Moorthy K.K., Babu S.S., Satheesh S.K. Aerosol cha-racteristics and radiative impacts over the Arabian Sea during the intermonsoon season: results from ARMEX field campaign // J. Atmos. Sci. 2005. V. 62. P. 192–206.
  14. Moorthy K.K., Saha A., Prasad B.S.N., Niranjan K., Jhurry D., Pillai P.S. Aerosol optical depths over peninsular India and adjoining oceans during the INDOEX campaigns: Spatial, temporal, and spectral characteristics // J. Geophys. Res. D. 2001. V. 106, N 22. P. 28,539–28,554.
  15. Satheesh S.K., Moorthy K.K., Murthy B.V.K. Spatial gradients in aerosol characteristics over the Arabian Sea and Indian Ocean // J. Geophys. Res. D. 1998. V. 103, N 20. P. 26,183–26,192.
  16. Moorthy K.K., Satheesh S.K., Baby S.S., Saha A. Large latitudinal gradients and temporal heterogeneity in aerosol black carbon and its mass mixing ratio over southern and northern oceans observed during a trans-continental cruise experiment // Geophys. Res. Lett. 2005. V. 32. L14818. DOI: 10.1029/2005GL023267.
  17. Moorthy K.K., Satheesh S.K., Murthy B.V.K. Investigations of marine aerosols over the tropical Indian Ocean // J. Geophys. Res. D. 1997. V. 102, N 15. P. 18827–18842.
  18. Prakash P.J., Stenchikov G., Tao W., Yapici T., Warsama B., Engelbrecht J. Study of Arabian Red Sea coastal soils as potential mineral dust sources // Atmos. Chem. Phys. 2016. V. 16, N 18. P. 11991–12004. URL: http://www.atmos-chem-phys.net/ 16/11991/2016/ DOI: 10.5194/acp-16-11991-2016.
  19. Abdallah R.I., Khalil N.M., Roushdie M.I. Monitoring of pollution in Egyptian Red Sea // Egyptian Journal of Petroleum. 2015. V. 24. P. 59–70.
  20. Badarinath K.V.S., Kharol S.K., Sharma A.R. Long-range transport of aerosols from agriculture crop residue burning in Indo-Gangetic Plains e a study using LIDAR, ground measurements and satellite data // J. Atmos. Solar-Terr. Phys. 2009. V. 71. P. 112–120.
  21. Dey S., Di Girolamo L. A climatology of aerosol optical and microphysical properties over the Indian subcontinent from 9 years (2000–2008) of Multiangle Imaging Spectroradiometer (MISR) data // J. Geophys. Res. 2010. V. 115. D15204. DOI: 10.1029/ 2009JD013395.
  22. Duflot V., Royer P., Chazette P., Baray J.-L., Courcoux Y., Delmas R. Marine and biomass burning aerosols in the southern Indian Ocean: retrieval of aerosol optical properties from ship-borne lidar and sun-photometer measurements // J. Geophys. Res. 2011. V. 116. D18208. DOI: 10.1029/2011JD015839.
  23. Pol'kin V.V., Kabanov D.M., Sakerin S.M., Golobokova L.P. Rezul'taty sravnitel'nyh issledovanij opticheskih, mikrofizicheskih harakteristik i himicheskogo sostava ajerozolja nad Kaspijskim morem v 26-m i 41-m rejsah NIS «Rift» // Optika atmosf. i okeana. 2013. V. 26, N 8. P. 628–635; Pol’kin V.V., Kabanov D.M., Sakerin S.M., Golobokova L.P. Comparative studies of optical and microphysical characteristics and chemical xomposition of aerosol over water basin of Caspian Sea in the 29th and 41st cruises of RV Rift // Atmos. Ocean. Opt. 2014. V. 27, N 1. P. 16–23.
  24. Sakerin S.M., Kabanov D.M., Pol'kin V.V., Radionov V.F., Holben B.N., Smirnov A. Variacii opticheskih i mikrofizicheskih harakteristik ajerozolja na marshrute Rossijskih antarkticheskih jekspedicij v Vostochnoj Atlantike // Optika atmosf. i okeana. 2016. V. 29, N 8. P. 666–678. DOI: 10.15372/ AOO20160808.
  25. Sakerin S.M., Kabanov D.M., Rostov A.P., Turchinovich S.A., Knjazev V.V. Solnechnye fotometry dlja izmerenij spektral'noj prozrachnosti atmosfery v stacionarnyh i mobil'nyh uslovijah // Optika atmosf. i okeana. 2012. V. 25, N 12. P. 1112–1117; Sakerin S.M., Kabanov D.M., Rostov A.P., Turchinovich S.A., Knyazev V.V. Sun photometers for measuring spectral air transparency in stationary and mobile conditions // Atmos. Ocean. Opt. 2013. V. 26, N 4. P. 352–356.
  26. Schetchik ajerozol'nyh chastic AZ-10. Rukovodstvo po jekspluatacii. JeKIT 7.830.000 RJe. M., 2010. 13 p.
  27. Kozlov V.S., Shmargunov V.P., Pol'kin V.V. Spektrofotometry dlja issledovanija harakteristik pogloshhenija sveta ajerozol'nymi chasticami // Pribory i tehn. jeksperim. 2008. N 5. P. 155–157.
  28. Sakerin S.M., Kabanov D.M. Melko- i grubodispersnye komponenty ajerozol'noj opticheskoj tolshhi atmosfery v morskih i poljarnyh rajonah // Optika atmosf. i okeana. 2015. V. 28, N 8. P. 690–697; Sakerin S.M., Kabanov D.M. Fine and coarse components of atmospheric aerosol optical depth in maritime and polar regions // Atmos. Ocean. Opt. 2015. V. 28, N 6. P. 510–517.
  29. Acker J.G., Leptoukh G. Online Analysis Enhances Use of NASA Earth Science Data // Eos, Trans. AGU. 2007. V. 88, N 2. P. 14–17.
  30. URL: http://giovanni.sci.gsfc.nasa.gov
  31. Poddubnyj V.A., Pol'kin V.V., Sakerin S.M., Golobokova L.P., Luzheckaja A.P., Markelov Ju.I., Dubinkina E.S., Huriganova O.I. Kompleksnyj ajerozol'nyj jeksperiment na Srednem Urale. Part 1. Uslovija provedenija i rezul'taty fotometricheskih izmerenij // Optika atmosf. i okeana. 2016. V. 29, N 12. P. 1003–1010.
  32. Kalapureddy M.C.R., Kaskaoutis D.G., Raj P. Ernest, Devara P.C.S., Kambezidis H.D., Kosmopoulos P.G., Nastos P.T. Identification of aerosol type over the Arabian Sea in the remonsoon season during the Integrated Campaign for Aerosols, Gases and Radiation Budget (ICARB) // J. Geophys. Res. 2009. V. 114. D17203. DOI: 10.1029/2009JD011826.
  33. Pol'kin V.V., Shhelkanov N.N., Golobokova L.P., Panchenko M.V. Sravnenie metodik ocenki vklada kontinental'nyh i morskih istochnikov v ionnyj sostav privodnogo ajerozolja Belogo morja // Optika atmosf. i okeana. 2008. V. 21, N 1. P. 23–26.
  34. Kondrat'ev K.Ja. Ajerozol' i klimat. L.: Gidrometeoizdat, 1991. 541 p.
  35. Proemse B.C., Mayer B., Fenn M.E. Tracing industrial sulfur contributions to atmospheric sulfate deposition in the Athabasca oil sands region, Alberta, Canada // Appl. Geochem. 2012. V. 27. P. 2425–2434.