The volume concentration of fine and coarse aerosol (Vf and Vс) in the near-water layer and the aerosol optical depth (AOD) of the atmosphere are generalized on the basis of long-term studies in Eurasian sector of the Arctic ocean. The mean AOD value at 0.5 mm is 0.061, the Angstrom exponent is 0.9, the concentrations of fine and coarse aerosol are 0.35 and 2.5 mm3/cm3, respectively. The greatest content of fine aerosol is observed in the atmosphere over Norwegian and Barents Seas. The spatial distribution is characterized by the decrease in the concentrations in northern and eastern directions: the mean value Vf becomes 1.7 times less from Barents Sea to Chukchi Sea (from 0,43 to 0.26 mm3/cm3). The very high concentration of coarse aerosol are observed in south-east part of Kara Sea: the mean Vс is 4.18 mm3/cm3. Then the coarse aerosol concentration decreases relatively to Kara Sea in eastern and western directions by several times.
Arctic, sea expeditions, aerosol concentrations, aerosol optical depth, spatial distribution
1. Physics and Chemistry of the Arctic Atmosphere / A. Kokhanovsky, C. Tomasi (eds.). England: Springer Polar Sciences series, 2020. 717 p. DOI: ORG/10.1007/978-3-030-33566-3.
2. Abbatt J.P.D., Leaitch W.R., Aliabadi A.A., Bertram A.K., Blanchet J.-P., Boivin-Rioux A., Bozem H., Burkart J., Chang R.Y.W., Charette J., Chaubey J.P., Christensen R.J., Cirisan A., Collins D.B., Croft B., Dionne J., Evans G.J., Fletcher C.G., Gal M., Ghahremaninezhad R., Girard E., Gong W., Gosselin M., Gourdal M., Hanna S.J., Hayashida H., Herber A.B., Hesaraki S., Hoor P., Huang L., Hussherr R., Irish V.E., Keita S.A., Kodros J.K., Kollner F., Kolonjari F., Kunkel D., Ladino L.A., Law K., Levasseur M., Libois Q., Liggio J., Lizotte M., Macdonald K.M., Mahmood R., Martin R.V., Mason R.H., Miller L.A., Moravek A., Mortenson E., Mungall E.L., Murphy J.G., Namazi M., Norman A.-L., O'Neill N.T., Pierce J.R., Russell L.M., Schneider J., Schulz H., Sharma S., Si M., Staebler R.M., Steiner N.S., Thomas J.L., von Salzen K., Wentzell J.J.B., Willis M.D., Wentworth G.R., Xu J.-W., Yakobi-Hancock J.D. Overview paper: New insights into aerosol and climate in the Arctic // Atmos. Chem. Phys. 2019. V. 19, N 4. P. 2527–2560. DOI: 10.5194/acp-19-2527-2019.
3. Xian P., Zhang J., O’Neill N.T., Toth T.D., Sorenson B., Colarco P.R., Kipling Z., Hyer E.J., Campbell JR., Reid J.S., Ranjbar K. Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 1: Climatology and trend // Atmos. Chem. Phys. 2022. V. 22, N 15. P. 9915–9947. DOI: 10.5194/acp-22-9915-2022.
4. Kabanov D.M., Maslovsky A.S., Radionov V.F., Sakerin S.M., Chernov D.G., Sidorova O.R. Sezonnaya i mezhgodovaya izmenchivost' kharakteristik aerozolya po dannym mnogoletnikh (2011–2021 years) izmerenii v Rossiiskom nauchnom tsentre na arkhipelage Shpitsbergen // Optika atmosf. i okeana. 2023. V. 36, N 6. P. 433–442. DOI: 10.15372/AOO20230602; Kabanov D.M., Maslovsky A.S., Radionov V.F., Sakerin S.M., Sidorova O.R., Chernov D.G. Seasonal and interannual variability of aerosol characteristics according to the data of long-term (2011–2021) measurements at the Russian Scientific Center on the Spitzbergen Archipelago // Atmos. Ocean. Opt. 2023. V. 36, N 6. P. 645–654.
5. Sakerin S.M., Kabanov D.M., Loskutova M.A., Rize D.D., Cрernov D.G., Turchinovich Yu.S. Kharakteristiki aerozolya na nauchno-issledovatel'skom statsionare «Ledovaya baza “Mys Baranova”» v 2018–2023 years // Problemy Arktiki i Antarktiki. 2023. V. 69, N 4. P. 421–434. DOI: 10.30758/0555-2648-2023-69-4-421-434.
6. Asmi E., Kondratyev V., Brus D., Laurila T., Lihavainen H., Backman J., Vakkari V., Aurela M., Hatakka J., Viisanen Y., Uttal T., Ivakhov V., Makshtas A. Aerosol size distribution seasonal characteristics measured in Tiksi, Russian Arctic // Atmos. Chem. Phys. 2016. V. 16. P. 1271–1287. DOI: 10.5194/acp-16-1271-2016.
7. Xing J., Bian L., Hu Q., Yu J., Sun C., Xie Z. Atmospheric black carbon along a cruise path through the Arctic Ocean during the Fifth Chinese Arctic Research Expedition // Atmosphere. 2014. V. 5. P. 292–306. DOI: 10.3390/atmos5020292.
8. Ferrero L., Sangiorgi G., Perrone M.G., Rizzi C., Cataldi M., Markuszewski P., Pakszys P., Makuch P., Petelski T., Becagli S., Traversi R., Bolzacchini E., Zielinski T. Chemical composition of aerosol over the Arctic Ocean from summer ARcticEXpedition (AREX) 2011–2012 cruises: Ions, amines, elemental carbon, organic matter, polycyclic aromatichydrocarbons, n-Alkanes, metals, and rare Earth elements // Atmosphere. 2019. V. 10, N 54. DOI: 10.3390/atmos10020054.
9. Park J., Dall’Osto M., Park K., Gim Y., Kang H.J., Jang E., Park K.-T., Park M., Yum S.S., Jung J., Lee B.Y., Yoon Y.J. Shipborne observations reveal contrasting Arctic marine, Arctic terrestrial and Pacific marine aerosol properties // Atmos. Chem. Phys. 2020. V. 20, N 5. P. 5573–5590. DOI: 10.5194/acp-20-5573-2020.
10. Sakerin S.M., Kabanov D.M., Makarov V.I., Polkin V.V., Popova S.A., Chankina O.V., Pochufarov A.O., Radionov V.F., Rize D.D. Spatial distribution of atmospheric aerosol physicochemical characteristics in Russian sector of the Arctic Ocean // Atmosphere. 2020. V. 11, N 11. P. 1170. DOI: 10.3390/atmos1111170.
11. Antokhina O.Yu., Antokhin P.N., Arshinova V.G., Arshinov M.Yu., Belan B.D., Belan S.B., Davydov D.K., Ivlev G.A., Kozlov A.V., Nédélec Ph., Paris J.-D., Rasskazchikova T.M., Savkin D.E., Simonenkov D.V., Sklyadneva T.K., Tolmachev G.N., Fofonov A.V. Vertikal'noe raspredelenie gazovykh i aerozol'nykh primesei vozdukha nad rossiiskim sektorom Arktiki // Optika atmosf. i okeana. 2017. V. 30, N 12. P. 1043–1052. DOI: 10.15372/AOO20171207; Antokhina O.Yu., Antokhin P.N., Arshinova V.G., Arshinov M.Yu., Belan B.D., Belan S.B., Davydov D.K., Ivlev G.A., Kozlov A.V., Nédélec P., Paris J.-D., Rasskazchikova T.M., Savkin D.E., Simonenkov D.V., Sklyadneva T.K., Tolmachev G.N., Fofonov A.V. Vertical distributions of gaseous and aerosol admixtures in air over the Russian Arctic // Atmos. Ocean. Opt. 2018. V. 31, N 3. P. 300–310.
12. Zenkova P.N., Chernov D.G., Shmargunov V.P., Panchenko M.V., Belan B.D. Submikronnyi aerozol' i pogloshchayushchee veshchestvo v troposfere rossiiskogo sektora Arktiki po dannym izmerenii samoleta-laboratorii Tu-134 «Optik» v 2020 year // Optika atmosf. i okeana. 2021. V. 34, N 11. P. 882–890. DOI: 10.15372/AOO20211108; Zenkova P.N., Chernov D.G., Shmargunov V.P., Panchenko M.V., Belan B.D. Submicron aerosol and absorbing substance in the troposphere of the Russian Sector of the Arctic according to measurements onboard the Tu-134 Optik aircraft laboratory in 2020 // Atmos. Ocean. Opt. 2022. V. 35, N 1. P. 43–51.
13. Antokhina O.Yu., Antokhin P.N., Arshinova V.G., Arshinov M.Yu., Belan B.D., Belan S.B., Berdashkinova O.I., Golobokova L.P., Davydov D.K., Ivlev G.A., Kozlov A.V., Onishchuk N.A., Rasskazchikova T.M., Savkin D.E., Simonenkov D.V., Sklyadneva T.K., Tolmachev G.N., Fofonov A.V., KHodzher T.V. Sostav vozdukha nad Rossiiskim sektorom Arktiki v sentyabre 2020 year 4. Atmosfernyi aerozol' // Optika atmosf. i okeana. 2024. V. 37, N 3. P. 214–224. DOI: 10.15372/AOO20240305.
14. Glantz P., Bourassa A., Herber A., Iversen T., Karlsson J., Kirkevåg A., Maturilli M., Seland Ø., Stebel K., Struthers H., Tesche M., Thomason L. Remote sensing of aerosols in the Arctic for an evaluation of global climate model simulations // J. Geophys. Res.: Atmos. 2014. V. 119. P. 8169–8188. DOI: 10.1002/2013JD021279.
15. Hsu N.C., Gautam R., Sayer A.M., Bettenhausen C., Li C., Jeong M.J., Tsay S.-C., Holben B.N. Global and regional trends of aerosol optical depth over land and ocean using SeaWiFS measurements from 1997 to 2010 // Atmos. Chem. Phys. 2012. V. 12. P. 8037–8053. DOI: 10.5194/acp-12-8037-2012.
16. Markowicz K.M., Pakszys P., Ritter C., Zielinski T., Udisti R., Cappelletti D., Mazzola M., Shiobara M., Xian P., Zawadzka O., Lisok J., Petelski T., Makuch P., Karasiński G. Impact of North American intense fires on aerosol optical properties measured over the European Arctic in July 2015 // J. Geophys. Res.: Atmos. 2016. V. 121. P. 14,487–14,512. DOI: 10.1002/2016JD025310.
17. Remer L.A., Kaufman Y.J., Tanre D., Mattoo S., Chu D.A., Martins J.V., Li R.-R., Ichoku C., Levy R.C., Kleidman R.G., Eck T.F., Vermote E., Holben B.N. The MODIS aerosol algorithm, products, and validation // J. Atmos. Sci. 2005. V. 62, N 4. P. 947–973. DOI: 10.1175/JAS3385.1.
18. Gelaro R., McCarty W., Suárez M.J., Todling R., Molod A., Takacs L., Randles C.A., Darmenov A., Bosilovich M.G., Reichle R., Wargan K., Coy L., Cullather R., Draper C., Akella S., Buchard V., Conaty A., da Silva A.M., Gu W., Kim G.-K., Koster R., Lucchesi R., Merkova D., Nielsen J.E., Partyk G., Pawson S., Putman W., Rienecker M., Schubert S.D., Sienkiewicz M., Zhao B. The Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) // J. Climate. 2017. V. 30, N 14. P. 5419–5454. DOI: 10.1175/JCLI-D-16-0758.1.
19. Global Modeling and Assimilation Office (GMAO), 2015a. MERRA-2 tavgM_2d_aer_Nx: 2d, Monthly mean, Time-averaged, Single-Level, Assimilation, Aerosol Diagnostics V5.12.4, Greenbelt, MD, USA, Goddard Earth Sciences Data and Information Services Center (GES DISC). DOI: 10.5067/FH9A0MLJPC7N (last access: 15.04.2023).
20. Global Modeling and Assimilation Office (GMAO), 2015b. MERRA-2 tavg1_2d_aer_Nx: 2d, 1-Hourly, Time-averaged, Single-Level, Assimilation, Aerosol Diagnostics V5.12.4, Greenbelt, MD, USA, Goddard Earth Sciences Data and Information Services Center (GES DISC). DOI: 10.5067/KLICLTZ8EM9D (last access: 15.04.2023).
21. Mei L., Xue Y., de Leeuw G., von Hoyningen-Huene W., Kokhanovsky A.A., Istomina L., Guang J., Burrows J.P. Aerosol optical depth retrieval in the Arctic region using MODIS data over snow // Remote Sens. Environ. 2013. V. 128. P. 234–245. DOI: 10.1016/j.rse.2012. 10.009.
22. Zhuravleva T.B., Artyushina A.V., Vinogradova A.A., Voronina Yu.V. Chernyi uglerod v prizemnoi atmosfere vdali ot istochnikov emissii: sravnenie rezul'tatov izmerenii i reanaliza MERRA-2 // Optika atmosf. i okeana. 2020. V. 33, N 4. P. 250–260. DOI: 10.15372/AOO20200402; Zhuravleva T.B., Artyushina A.V., Vinogradova A.A., Voronina Yu.V. Black carbon in the near-surface atmosphere far away from emission sources: Comparison of measurements and MERRA-2 reanalysis data // Atmos. Ocean. Opt. 2020. V. 33, N 6. P. 591–601.
23. Turchinovich Yu.S., Pochufarov A.O., Sakerin S.M. Algorithm of controlling the quality and retrieval of data from measurements of aerosol and black carbon concentrations in marine expeditions // Proc. SPIE. 2021. V. 11916. P. 119161U. DOI: 10.1117/12.2600591.
24. Chen Y.-C., Hamre B., Frette Q., Muyimbwa D., Blindheim S., Stebel K., Sobolewski P., Toledano C., Stamnes J. Aerosol optical properties in Northern Norway and Svalbard // Appl. Opt. 2016. V. 55, N 4. DOI: 10.1364/AO.55.000660.
25. Smithsonian Institution – Global Volcanism Program: Worldwide Holocene Volcano and Eruption Information. URL: https://volcano.si.edu (last access: February 2022).
26. Sakerin S.M., Kabanov D.M., Kopeikin V.M., Kruglinsky I.A., Novigatsky A.N., Shevchenko V.P., Turchinovich Yu.S. Spatial distribution of atmospheric black carbon in the Eurasian sector of the Arctic Ocean from 28 marine expeditions (2007–2022) // Atmos. Pollut. Res. 2023. V. 14. P. 101885. DOI: 10.1016/j.apr.2023.101885.