Vol. 26, issue 12, article # 7

Abstract:

The paper presents unique data of 12 years (2001–2012) monitoring at Klyuchi site (Novosibirsk region) on changes in aerosol mass concentrations and concentrations of organic carbon (ОС), elemental carbon (ЕС) and total protein (ТР) in it. It was found that aerosol mass concentrations, OC, and OC/ЕС ratio have trends to increase, but TP has a trend to decrease. Seasonal changes in observed EC, OC and TP concentrations and its ratios are also revealed. The comparison of data obtained and recently published data for other Asia and Europe regions show that there are good agreements between them for some regions and no agreement for some other regions.

Keywords:

atmospheric aerosol, organic/elemental carbon, bioaerosols, monitoring

References:

1. Hidy G.M. Aerosols. An industrial and environmental science. Orlando: Academic Press, 1984. 774 p.
2. Himija okruzhajushhej sredy / Pod red. O.M. Bokrisa. M.: Himija, 1978. 672 p.
3. Pio C., Cerqueira M., Harrison R.V., Nunes T., Mirante F., Alves C., Oliveira C., Sanchez de la Campa A., Artiñano B., Matos M. OC/EC ratio observations in Europe: Re-thinking the approach for appointment between primary and secondary organic carbon // Atmos. Environ. 2011. V. 45, N 34. P. 6121–6132.
4. Cheng Y., He K.-B., Duan F.-K., Zheng M., Du Z.-Y., Ma Y.-L., Tan J.-H. Ambient organic carbon to elemental carbon ratios: Influences of the measurement methods and implications // Atmos. Environ. 2011. V. 45, N 12. P. 2060–2066.
5. Grivas G., Cheristandis S., Chaloulakou A. Elemental and organic carbon in the urban environment of Athens. Seasonal and diurnal variations and estimates of secondary organic carbon // Sci. Total. Environ. 2012. V. 414. P. 535–545. doi: 10.1016/j.scitotenv.2011.10.058.
6. Després V.R., Huffman J.A., Burrows S.M., Hoose C., Safatov A.S., Buryak G.A., Fröhlich-Nowoisky J., Elbert W., Andreae M.O., Pöschl U., Jaenicke R. Primary biological aerosols in the atmosphere: Observations and relevance // Tellus B. Chem. Phys. Meteorol. 2012. V. 64. P. 1–58. doi: 10.3402/tellusb.v64i0.15598.
7. Safatov A.S., Buryak G.A., Andreeva I.S., Olkin S.E., Reznikova I.K., Sergeev A.N., Belan B.D., Panchenko M.V. Atmospheric bioaerosols // Aerosols – Science and Technology / Ed. I. Agranovski. Weinheim: Wiley – VCH, 2010. P. 407–454.
8. Уорк К., Уорнер С. Загрязнение воздуха. Источники и контроль. М.: Мир, 1980. 640 с.
9. Berljand M.E. Prognoz i regulirovanie zagrjaznenija atmosfery. L.: Gidrometeoizdat, 1985. 271 p.
10. Viana M., Reche C., Amato F., Alastuey A., Querol X., Moreno T., Lucarelli F., Nava S., Cazolai G., Chiari M., Rico M. Evidence of biomass burning aerosols in the Barcelona urban environment during winter time // Atmos. Environ. 2013. V. 72. P. 81–88. URL: http://dx.doi. org/10.1016/j.atmosenv.2013.02.031
11. Keuken M.P., Moerman M., Voogt M., Blom M., Weijers E.P., Röckmann T., Dusek U. Source contributions to PM2.5 and PM10 at an urban background and a street location // Atmos. Environ. 2013. V. 71. P. 26–35. URL: http://dx.doi.org/10.1016/j.atmosenv.2013.01.032
12. Saud T., Saxena M., Singh D.P., Saraswati, Dahiya M., Sharma S.K., Datta A., Gadi R., Mandal T.K. Spatial variation of chemical constituents from the burning of commonly used biomass fuels in rural areas of the Indo-Gangetic Plain (IGP), India // Atmos. Environ. 2013. V. 71. P. 158–169. URL: http://dx.doi.org/10.1016/j. atmosenv. 2013.01.053
13. Zhao P., Dong F., Yang Y., He D., Zhao X., Zhang W., Yao Q., Liu H. Characteristics of carbonaceous aerosol in the region of Beijing, Tianjin, and Hebei, China // Atmos. Environ. 2013. V. 71. P. 389–398. URL: http: //dx.doi.org/10.1016/j.atmosenv.2013.02.010
14. Gianini M.F.D., Piot C., Herich H., Besombes J.-L., Jaf-frezo J.-L., Hueglin C. Source apportionment of PM10, organic carbon and elemental carbon at Swiss sites: An intercomparison of different approaches // Sci. Total Environ. 2013. V. 454–455. P. 99–108. doi: 10.1016/ j.scitotenv.2013.02.043.
15. Caserini S., Galante S., Ozgen S., Cucco S., de Gregorio K., Moretti M. A methodology for elemental and organic carbon emission inventory and results for Lombardy region, Italy // Sci. Total Environ. 2013. V. 450–451. P. 22–30. doi: 10.1016/j.scitotenv.2013.01.073.
16. Popova S.A., Makarov V.I., Bashenhaeva N.V., Hodzher T.V. Sravnenie rezul'tatov izmerenija soderzhanija ugleroda v atmosfernyh ajerozoljah metodami reakcionnoj gazovoj hromatografii i suhogo sozhzhenija // Himija v interesah ustojchivogo razvitija. 2007. V. 15, N 1. P. 97–103.
17. Bizin M.A., Popova S.A., Chankina O.V., Makarov V.I., Shinkorenko M.P., Smoljakov B.S., Kucenogij K.P. Vlijanie lesnyh pozharov na massovuju koncentraciju, dispersnyj i himicheskij sostav atmosfernogo ajerozolja v regional'nom masshtabe // Optika atmosf. i okeana. 2013. V. 26, N 6. P. 484–489.
18. You W.W., Haugland R.P., Ryan D.K., Haugland R.P. 3-(4-Carboxybenzoyl)quinoline-2-carboxaldehyde, a reagent with broad dynamic range for the assay of proteins and lipoproteins in solution // Annal. Biochem. 1997. V. 244, N 2. P. 277–282.
19. Kozlov V.S., Panchenko M.V., Jausheva E.P. Vremennaja izmenchivost' soderzhanija submikronnogo ajerozolja i sazhi v prizemnom sloe atmosfery Zapadnoj Sibiri // Optika atmosf. i okeana. 2007. V. 20, N 12. P. 1082–1085.
20. Kozlov V.S., Panchenko M.V., Jausheva E.P. Submikronnyj ajerozol' i sazha prizemnogo sloja v sutochnom hode // Optika atmosf. i okeana. 2010. V. 23, N 7. P. 561–569.