Vol. 32, issue 06, article # 2

Vinogradova A. A., Kopeikin V. M., Smirnov N. S., Vasilieva A. V., Ivanova Yu. A. Black carbon in surface air in the Pechora-Ilych nature reserve: measurements and sources. // Optika Atmosfery i Okeana. 2019. V. 32. No. 06. P. 430–436. DOI: 10.15372/AOO20190602 [in Russian].
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Abstract:

The new data on the surface atmospheric black carbon (BC) concentration derived from continuous daily sampling during October 2017 – March 2018, that is, cold half year without wildfires as BC sources, in the remote area of Pechora-Ilych Nature Biosphere Reserve are analyzed. Average BC concentrations (with standard deviations) are equal to (296 ± 172) and (175 ± 82) ng/m3 for settlement Yaksha and in its neighborhood, respectively. Monthly average BC concentrations measured are compared with related monthly average satellite data (https://giovanni.gsfc.nasa.gov/giovanni/). A good agreement between them may be regarded as their inter-calibration and confirms the reliability of both result types. The analysis of air mass trajectories at the observation point shows the main anthropogenic BC sources to be situated at a distances of less than 500 km in industrial areas of the Central Urals, gas and oil production areas of Yamalo-Nenets and Khanty-Mansiysk Autonomous District, towns and settlements of Perm region, Udmurtia, and Komi Republic.

Keywords:

atmosphere, surface layer, Pechora-Ilych nature reserve, black carbon

References:

  1. AMAP Assessment 2015: Black carbon and ozone as Arctic climate forcers. Oslo, Norway: Arctic Monitoring and Assessment Programme, 2015. 116 p.
  2. Panchenko M.V., Zhuravleva T.B., Kozlov V.S., Nasrtdinov I.M., Pol'kin V.V., Terpugova S.A., Chernov D.G. Otsenka radiatsionnykh effektov aerozolya v fonovykh i zadymlennykh usloviyakh atmosfery Sibiri na osnove empiricheskikh dannykh // Meteorol. i gidrol. 2016. N 2. P. 45–54.
  3. Bond T.C., Doherty S.J., Fahey D.W., Forster P.M., Berntsen T., DeAngelo B.J., Flanner M.G., Ghan S., Kärcher B., Koch D., Kinne S., Kondo Y., Quinn P.K., Sarofim M.C., Schultz M.G., Schulz M., Venkataraman C., Zhang H., Zhang S., Bellouin N., Guttikunda S.K., Hopke P.K., Jacobson M.Z., Kaiser J.W., Klimont Z., Lohmann U., Schwarz J.P., Shindell D., Storelvmo T., Warren S.G., Zender C.S. Bounding the role of black carbon in the climate system: A scientific assessment // J. Geophys. Res. Atmos. 2013. V. 118. P. 5380–5552.
  4. Schmeisser L., Backman J., Ogren J.A., Andrews E., Asmi E., Starkweather S., Uttal T., Fiebig M., Sharma S., Eleftheriadis K., Vratolis S., Bergin M., Tunved P., Jefferson A. Seasonality of aerosol optical properties in the Arctic // Atmos. Chem. Phys. 2018. V. 18. P. 11599–11622.
  5. Kopejkin V.M. Nablyudeniye sazhevogo aerozolya v atmosfere nad Rossiyej v mezhdunarodnykh ekspeditsiyakh TROICA // Optika atmosf. i okeana. 2007. V. 20, N 7. P. 641–646.
  6. Yemilenko A.S., Kopejkin V.M. Sravneniye sinkhronnykh izmerenij kontsentratsii sazhi i submikronnogo aerozolya v regionakh s razlichnoj stepen'yu antropogennoj nagruzki // Optika atmosf. i okeana. 2009. V. 22, N 6. P. 535–540; Emilenkо А.S., Kоpeikin V.М. Comparison of synchronous measurements of soot and submicron aerosol concentrations in regions with different anthropogenic loadings // Atmos. Ocean. Opt. 2009. V. 22, N 4. P. 421–427.
  7. Limon-Sanchez M.T., Carbajal-Romero P., Hernandez-Mena L., Saldarriaga-Norena H., Lopez-Lopez A., Cosio-Ramirez R., Arriaga-Colina J.L., Smith W. Black carbon in PM2.5, data from two urban sites in Guadalajara, Mexico during 2008 // Atmos. Pollut. Res. 2011. V. 2. P. 358–365. DOI: 10.5094/APR.2011.040.
  8. Kopejkin V.M., Yemilenko A.S., Isakov A.A., Loskutova O.V., Ponomareva T.YA. Izmenchivost' sazhevogo i submikronnogo aerozolya v Moskovskom regione v 2014–2016 years. // Optika atmosf. i okeana. 2018. V. 31, N 1. P. 5–10; Kоpeikin V.М., Emilenkо А.S., Isakov А.А., Lоskutovа О.V., Pоnomarevа Т.Ya. Variability of soot and fine aerosol in the Moscow Region in 2014–2016 // Atmos. Ocean. Opt. 2018. V. 31, N 3. P. 243–249.
  9. Kozlov V.S., Panchenko M.V., Yausheva Ye.P. Submikronnyj aerozol' i sazha prizemnogo sloya v sutochnom khode // Optika atmosf. i okeana. 2010. V. 23, N 7. P. 561–569; Kоzlov V.S., Pаnchenkо М.V., Yaushevа Е.P. Diurnal variations of the submicron aerosol and black carbon in the near-ground layer // Atmos. Ocean. Opt. 2011. V. 24, N 1. P. 30–38.
  10. Makshtas A.P., Uttal T., Laurilla T., Paramonova N.A. Gidrometeorologicheskaya observatoriya Tiksi (k pyatiletiyu otkrytiya) // Problemy Arktiki i Antarktiki. 2015. N 2 (104). P. 5–12.
  11. Popovicheva O., Diapouli E., Makshtas A., Shonija N., Manousakas M., Saraga D., Uttae T., Eleftheriadis K. East Siberian Arctic background and black carbon polluted aerosols at HMO Tiksi // Sci. Total Environ. 2019. V. 655. P. 924–938. DOI: 10.1016/j.scitotenv.2018.11.165.
  12. Kopejkin V.M., Repina I.A., Grechko Ye.I., Ogorodnikov B.I. Izmereniye soderzhaniya sazhevogo aerozolya nad vodnoj poverkhnost'yu v YUzhnom i Severnom polushariyakh // Optika atmosf. i okeana. 2010. V. 23, N 6. P. 444–450; Kоpeikin V.М., Repinа I.A., Grechkо Е.I., Оgorodnikov B.I. Measurements of soot aerosol content in the near-water atmospheric layer in the southern and northern hemispheres // Atmos. Ocean. Opt. 2010. V. 23, N 6. P. 500–507.
  13. Kozlov V.S., Shmargunov V.P., Panchenko M.V. Sezonnaya izmenchivost' vertikal'nykh profilej pogloshchayushchikh kharakteristik submikronnogo aerozolya v troposfere // Optika atmosf. i okeana. 2009. Т. 22, № 7. С. 635–642.
  14. Doherty S.J., Warren S.G., Grenfell T.C., Clarke A.D., Brandt R.E. Light-absorbing impurities in Arctic snow // Atmos. Chem. Phys. 2010. V. 10. P. 11647–11680.
  15. Shevchenko V.P., Kutsenogij K.P., Makarov V.I., Panchenko M.V., Pol'kin V.V., Popova S.A., Novigatskij A.N. Aerozoli // Sistema Belogo morya. V. II. Vodnaya tolshcha i vzaimodejstvuyushchiye s nej atmosfera, kriosfera, rechnoj stok i biosfera. M.: Nauchnyj mir, 2012. P. 50–69.
  16. Acker J.G., Leptoukh G. Online analysis enhances use of NASA Earth science data // Eos., Trans. AGU. V. 88, N 2. Р. 14–17.
  17. Hansen A.D.A., Rosen H., Novakov T. The aethalometer–an instrument for real-time measurement of optical absorption by aerosol particles // Sci. Total. Environ. 1984. V. 36, N 1. P. 191–196.
  18. Vinogradova A.A. Distantsionnaya otsenka vliyaniya zagryazneniya atmosfery na udalennyye territorii // Geofizicheskiye protsessy i biosfera. 2014. V. 13, N 4. P. 5–20.
  19. Air Quality Engineering & Climate Studies Research Group [Electronic resource]. URL: http://acs.engr.utk.edu/Data.php (last access: 11.02.2019).
  20. Air Resources Laboratory [Electronic resource]. URL: https://www.arl.noaa.gov (last access: 11.02.2019).
  21. Huang K., Fu J.S., Prikhodko V.Y., Storey J.M., Romanov A., Hodson E.L., Cresko J., Morozova I., Ignatieva Y., Cabaniss J. Russian anthropogenic black carbon: Emission reconstruction and Arctic black carbon simulation // J. Geophys. Res. Atmos. 2015. V. 120. DOI: 10.1002/2015JD023358.
  22. Makarov V.A., Okhta S. Organicheskij i neorganicheskij uglerod v atmosfernykh aerozolyakh Yakutii // Optika atmosf. i okeana. 2004. V. 17, N 9. P. 774–778.
  23. Vinogradova A.A., Titkova T.B., Ivanova Yu.A. Epizody anomal'no vysokoj kontsentratsii chernogo ugleroda v prizemnom vozdukhe v rajone stantsii Tiksi, Yakutiya // Optika atmosf. i okeana. 2018. V. 31, N 10. P. 837–844; Vinogradovа А.А., Тitkovа Т.B., Ivanovа Yu.А. Episodes with anomalously high black carbon concentration in surface air in the region of Tiksi station, Yakutiya // Atmos. Ocean. Opt. 2019. V. 32, N 1. P. 94–102.
  24. Gong S.L., Zhao T.L., Sharma S., Toom-Sauntry D., Lavoué D., Zhang X.B., Laitch W.R., Barrie L.A. Identification of trends and interannual variability of sulfate and black carbon in the Canadian High Arctic: 1981–2007 // J. Geophys. Res. 2010. V. 115. DOI: 10.1029/2009JD012943.
  25. Wang Q., Jacob D.J., Fisher J.A., Mao J., Leibensperger E.M., Carouge C.C., Le Sager P., Kondo Y., Jimenez J.L., Cubison M.J., Doherty S.J. Sources of carbonaceous aerosols and deposited black carbon in the Arctic in winter–spring: Implications for radiative forcing // Atmos. Chem. Phys. 2011. V. 11. P. 12453–12473.
  26. Eleftheriadis K., Vratolis S., Nyeki S. Aerosol black carbon in the European Arctic: Measurements at Zeppelin station, Ny-Ålesund, Svalbard from 1998–2007 // Geophys. Res. Lett. 2009. V. 36. DOI: 10.1029/2008GL035741.
  27. Shevchenko V.P., Starodymova D.P., Vinogradova A.A., Lisitsyn A.P., Makarov V.N., Popova S.A., Sivonen V.V., Sivonen V.P. Elementnyj i organicheskij uglerod v atmosfernom aerozole nad severo-zapadnym poberezh'yem Kandalakshskogo zaliva Belogo morya // Dokl. RAN. 2015. V. 461, N 1. P. 1–5.
  28. Kozlov V.S., Tikhomirov A.B., Panchenko M.V., Shmargunov V.P., Pol'kin V.V., Sakerin S.M., Lisitsyn A.P., Shevchenko V.P. Opticheskiye i mikrofizicheskiye kharakteristiki aerozolya v privodnoj atmosfere Belogo morya po dannym odnovremennykh korabel'nykh i beregovykh izmerenij v avguste 2006 year. // Optika atmosf. i okeana. 2009. V. 22, N 8. P. 767–776; Kozlov V.S., Тikhomirov А.B., Panchenkо М.V., Shmargunov V.P., Pol’kin V.V., Sakerin S.М., Lisitzin А.P., Shevchenkо V.P. Optical and microphysical parameters of aerosol in the near-water atmosphere of the White Sea as assessed from the data of simultaneous ship-borne and coast-based measurements in August 2006 // Atmos. Ocean. Opt. 2009. V. 22, N 5. P. 517–526.
  29. Stohl A., Klimont Z., Eckhardt S., Kupiainen K., Shevchenko V.P., Kopeikin V.M., Novigatsky A.N. Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions // Atmos. Chem. Phys. 2013. V. 13, N 17. P. 8833–8855.
  30. Access NASA Earth Science Data [Electronic resource]. URL: https://giovanni.gsfc.nasa.gov/giovanni (last access: 11.02.2019).